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Študija magnetnih lastnosti antiferomagneta $\mathrm{Ba_9 Yb_2 Si_6 O_{24}}$ z elektronsko paramagnetno resonanco
ID Puc, Matej (Author), ID Zorko, Andrej (Mentor) More about this mentor... This link opens in a new window

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Abstract
Kvantni materiali, v katerih je med magnetnimi ioni prisotna močna frustracija, so potencialni kandidati za realizacijo kvantne spinske tekočine. To je stanje, v katerem se magnetni momenti atomov ne uredijo niti pri temperaturi $T = 0$, zaznamujejo pa ga nenavadne fizikalne lastnosti, kot so močne kvantne fluktuacije, kvantna prepletenost ter frakcijske spinske vzbuditve. Zaradi njihove potencialne uporabe v tehnologiji so kvantne spinske tekočine aktualno področje raziskav v fiziki trdne snovi. V zaključni nalogi je z metodo elektronske paramagnetne resonance analiziran antiferomagnet $\mathrm{Ba_9 Yb_2 Si_6 O_{24}}$, ki je eden od kandidatov za realizacijo takšnega stanja. Rezultati meritev ne kažejo nenadnih sprememb v spektru, ki bi namignile na magnetno ureditev materiala do temperature $T = 4 \mathrm{K}$. Energijski nivoji Yb$^{3+}$ ionov, ki narekujejo magnetne lastnosti tega kvantnega magneta, se v kristalnem polju razcepijo na Kramersove dublete. Iz širin spektra, ki imajo zaradi relaksacij preko Orbachovega procesa eksponentno temperaturno odvisnost, je bil izmerjen tudi energijski razcep med osnovnim in prvim vzbujenim Kramersovim dubletom.

Language:Slovenian
Keywords:elektronska paramagnetna resonanca, kvantna spinska tekočina, magnetizem, orbitalna vrtilna količina, spin, Zeemanova interakcija, Orbachov proces, izmenjalna interakcija, $\mathrm{Ba_9 Yb_2 Si_6 O_{24}}$
Work type:Final paper
Typology:2.11 - Undergraduate Thesis
Organization:FMF - Faculty of Mathematics and Physics
Year:2026
PID:20.500.12556/RUL-179209 This link opens in a new window
COBISS.SI-ID:267965699 This link opens in a new window
Publication date in RUL:07.02.2026
Views:314
Downloads:152
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Secondary language

Language:English
Title:Study of magnetic properties of $\mathrm{Ba_9 Yb_2 Si_6 O_{24}}$ with electron paramagnetic resonance
Abstract:
Quantum materials in which strong magnetic frustration exists among the magnetic ions are promising candidates for the realization of a quantum spin liquid. This exotic state is characterized by the absence of long-range magnetic order even at temperature $T = 0$, and by unusual physical properties such as strong quantum fluctuations, quantum entanglement, and fractionalized spin excitations. Due to their potential technological applications, quantum spin liquids have become an active and rapidly growing field of research in condensed matter physics. In this thesis, the antiferromagnet $\mathrm{Ba_9 Yb_2 Si_6 O_{24}}$, which is one of the candidates for the realization of such a state, is analyzed using the method of electron paramagnetic resonance. The measurements do not show any abrupt changes in the spectrum that would indicate magnetic ordering of the material down to a temperature of $T = 4 \mathrm{K}$. The energy levels of the Yb$^{3+}$ ions, which determine the magnetic properties of this quantum magnet, split into Kramers doublets in the crystal field. From the linewidths of the spectrum, which exhibit an exponential temperature dependence due to the Orbach process, the energy splitting between the ground and the first excited Kramers doublet was also determined.

Keywords:electron paramagnetic resonance, quantum spin liquid, magnetism, orbital angular momentum, spin, Zeeman interaction, Orbach process, exchange interaction, $\mathrm{Ba_9 Yb_2 Si_6 O_{24}}$

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