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Photoinduced nonequilibrium states in Mott insulators
ID Murakami, Yuta (Author), ID Golež, Denis (Author), ID Eckstein, Martin (Author), ID Werner, Philipp (Author)

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Abstract
The study of nonequilibrium phenomena in interacting lattice systems can provide new perspectives on correlation effects and information on metastable states of matter. Mott insulators are a promising class of systems for nonequilibrium studies since they exhibit exotic phenomena and complex phase diagrams upon doping and because a large Mott gap provides protection against fast thermalization and heating after photoexcitations. One can thus expect the emergence of interesting nonlinear responses, transient states, and photoinduced phases in Mott systems. This review provides a comprehensive overview of the current understanding of photoexcited Mott insulators by discussing excitation protocols, nonlinear optical responses, the underlying mechanisms governing photocarrier dynamics, and the pathways leading to photoinduced metastable states. The review focuses on recent theoretical progress, identifies the relevant underlying concepts, and links them to experimental observations. The review starts with a general discussion of field-induced nonequilibrium setups and an overview of key experiments that revealed characteristic properties of photoexcited Mott states, proceeds with an overview of the theoretical tools that have been developed to investigate these strongly correlated nonequilibrium states, and then analyzes Mott insulators driven out of equilibrium by static electric fields, periodic fields, and short laser pulses. The appearance of nonthermal electronic orders in photoexcited Mott systems, including nonthermal spin and orbital orders, $\eta$-pairing states, and novel types of excitonic orders, is also discussed.

Language:English
Keywords:condensed matter physics, Mott insulators, strongly correlated systems, nonequilibrium systems, light-matter interaction, photoinduced transitions
Work type:Article
Typology:1.02 - Review Article
Organization:FMF - Faculty of Mathematics and Physics
Publication version:Author Accepted Manuscript
Year:2025
Number of pages:Str. 035001-1-035001-63
Numbering:Vol. 97, iss. 3
PID:20.500.12556/RUL-177240 This link opens in a new window
UDC:538.9
ISSN on article:0034-6861
DOI:10.1103/tkjh-lr83 This link opens in a new window
COBISS.SI-ID:262118403 This link opens in a new window
Publication date in RUL:18.12.2025
Views:548
Downloads:233
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Record is a part of a journal

Title:Reviews of modern physics
Shortened title:Rev. mod. phys.
Publisher:American Physical Society
ISSN:0034-6861
COBISS.SI-ID:26281984 This link opens in a new window

Secondary language

Language:Slovenian
Keywords:fizika kondenzirane snovi, Mottovi izolatorji, močno korelirani sistemi, neravnovesni sistemi, interakcije svetloba-snov, fotoinducirani prehodi

Projects

Funder:ARIS - Slovenian Research and Innovation Agency
Project number:P1-0044
Name:Teorija trdnih snovi in statistična fizika

Funder:ARIS - Slovenian Research and Innovation Agency
Project number:J1-2455
Name:Modeliranje neravnovesnih kvantnih materialov na različnih skalah

Funder:EC - European Commission
Project number:724103
Name:Nonequilibrium dynamical mean-field theory: From models to materials
Acronym:MODMAT

Funder:SNSF - Swiss National Science Foundation
Project number:205602
Name:NCCR MARVEL: Materials’ Revolution: Computational Design and Discovery of Novel Materials (phase III)

Funder:Other - Other funder or multiple funders
Funding programme:Japan Society for the Promotion of Science
Project number:JP20K14412
Name:Theoretical study of nonequilibrium steady states in strongly correlated systems and ordered phases

Funder:Other - Other funder or multiple funders
Funding programme:Japan Society for the Promotion of Science
Project number:JP21H05017
Name:Establishment of strong light field photoscience in solids and application to materials science

Funder:Other - Other funder or multiple funders
Funding programme:Japan Society for the Promotion of Science
Project number:JP24H00191
Name:-

Funder:Other - Other funder or multiple funders
Funding programme:Japan Society for the Promotion of Science
Project number:JP25K07235
Name:-

Funder:Other - Other funder or multiple funders
Funding programme:Japan Science and Technology Agency
Project number:JPMJCR1901
Name:Optical functions through symmetry breaking driven by carrier-envelope phase control of light

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