A CFD study on optimization of mass transfer and light distribution in a photocatalytic reactor with immobilized photocatalyst on spheres

Jamil, Qasim (avtor), Rana, Khush Bakhat (avtor), Matoh, Lev (avtor)

This study explores the influence of flow velocity, sphere size, and inter-sphere distance on hydrodynamics and mass transfer in a photocatalytic reactor. The effects of two different light configurations on light distribution and degradation were also evaluated. A 2D computational fluid dynamics (CFD) model was developed to simulate the continuous flow photocatalytic reactor with TiO$_2$-coated spheres and validated with experimental measurements by observing the degradation of methyl orange. The experimental setup consists of a tube containing an equal number of TiO$_2$-coated glass spheres. The case with radiation from one wall shows a non-uniform light distribution compared with the case with radiation from both walls. The CFD simulations focused on analyzing the velocity streamlines and turbulence characteristics (turbulent kinetic energy (TKE) and turbulence dissipation rate (TDR)). These parameters showed significant variations in each studied case. The case with larger spheres reached the highest velocity of 38 m/s of the pollutant solution. The highest TKE and TDR values of 0.47 m$^2/s^2$ and 12.2 m$^2/s^2$, respectively, were also observed in the same case, indicating enhanced mixing and mass transfer to the catalyst surfaces, ultimately leading to a more efficient degradation process. The results show that an optimized design of photocatalytic reactors can significantly improve mass transfer and, thus, degradation efficiency.

• Jezik: Angleški jezik
• Ključne besede: photocatalysis, reactor design optimization, AOPs, CFD analysis, glass beads
• Vrsta gradiva: Članek v reviji
• Tipologija: 1.01 - Izvirni znanstveni članek
• Organizacija: FKKT - Fakulteta za kemijo in kemijsko tehnologijo ; FS - Fakulteta za strojništvo
• Status publikacije: Objavljeno
• Različica publikacije: Objavljena publikacija
• Leto izida: 2024
• Št. strani: 13 str.
• Številčenje: Vol. 16, iss. 13, [art.] 1828
• PID: 20.500.12556/RUL-159008
• UDK: 544.526.5:628.3:66
• ISSN pri članku: 2073-4441
• DOI: 10.3390/w16131828
• COBISS.SI-ID: 199998211
• Datum objave v RUL: 27.06.2024

Gradivo je del revije

• Naslov: Water
• Skrajšan naslov: Water
• Založnik: Molecular Diversity Preservation International - MDPI
• ISSN: 2073-4441
• COBISS.SI-ID: 36731653

Licence

• Licenca: CC BY 4.0, Creative Commons Priznanje avtorstva 4.0 Mednarodna
• Povezava: http://creativecommons.org/licenses/by/4.0/deed.sl
• Opis: To je standardna licenca Creative Commons, ki daje uporabnikom največ možnosti za nadaljnjo uporabo dela, pri čemer morajo navesti avtorja.

Sekundarni jezik

• Jezik: Slovenski jezik
• Ključne besede: fotokataliza, optimizacija zasnove reaktorja, AOP-ji, analiza CFD, stekleni biseri